| Title | Star As | Genre | Info |
|---|---|---|---|
| Netflix vs. the World | Himself | - | - |
| Jane Fonda in Five Acts | Himself | - | - |
| The Old Man & the Gun | Forrest Tucker | - | aka "The Old Man and the Gun" |
| Earth: One Amazing Day | Narrator (voice) | - | - |
| Our Souls at Night | Louis Waters | - | - |
| The Big Bang | Narrator (voice) | - | - |
| The Discovery | Thomas Harbor | - | - |
| The Newspaperman: The Life and Times of Ben Bradlee | Himself | - | - |
| Pete's Dragon | Dan Rather | - | - |
| The Natural: The Best There Ever Was | Roy Hobbs | - | - |
| A Walk in the Woods | Bill Bryson | - | - |
| Truth | Dan Rather | - | - |
| Captain America: The Winter Soldier | Agent Alexander Pierce | - | - |
| All Is Lost | Our Man | - | - |
| The Company You Keep | Jim Grant / Nick Sloan | - | - |
| Lions for Lambs | Professor Stephen Malley | - | - |
| Charlotte's Web | Ike the Horse (voice) | - | aka Schweinchen Wilbur und seine Freunde (Germany) |
| An Unfinished Life | Einar Gilkyson | - | - |
| The Clearing | Wayne Hayes | - | aka Anatomie einer Entfuhrung (Germany) |
| Spy Game | Nathan D. Muir | - | - |
| The Last Castle | Lt. Gen. Eugene Irwin | - | - |
| The Horse Whisperer | Tom Booker | - | - |
| Up Close & Personal | Warren Justice | - | - |
| Indecent Proposal | John Gage | - | - |
| Sneakers | Martin Bishop/Martin Brice | - | - |
| Havana | Jack Weil | - | - |
| Legal Eagles | Tom Logan | - | - |
| Out of Africa | Denys George Finch Hatton | - | - |
| The Natural | Roy Hobbs | - | - |
| Brubaker | Henry Brubaker | - | - |
| The Electric Horseman | Norman 'Sonny' Steele | - | - |
| A Bridge Too Far | Maj. Julian Cook | - | - |
| All the President's Men | Bob Woodward | - | - |
| The Great Waldo Pepper | Waldo Pepper | - | - |
| Three Days of the Condor | Joseph Turner/The Condor | - | - |
| The Great Gatsby | Jay Gatsby | - | - |
| The Sting | Johnny Hooker aka Kelly | - | - |
| The Way We Were | Hubbell | - | - |
| Jeremiah Johnson | Jeremiah Johnson | - | - |
| The Candidate | Bill McKay | - | - |
| The Hot Rock | John Archibald Dortmunder | - | aka How to Steal a Diamond in Four Uneasy Lessons |
| Little Fauss and Big Halsy | Halsy Knox | - | - |
| Butch Cassidy and the Sundance Kid | The Sundance Kid | - | - |
| Downhill Racer | David Chappellet | - | - |
| Tell Them Willie Boy Is Here | Deputy Sheriff Christopher 'Coop' Cooper | - | - |
| Barefoot in the Park | Paul Bratter | - | - |
| The Chase | Charlie 'Bubber' Reeves | - | - |
| This Property Is Condemned | Owen Legate | - | - |
| Inside Daisy Clover | Wade Lewis | - | - |
| Situation Hopeless... But Not Serious | Captain Hank Wilson | - | - |
| War Hunt | Pvt. Roy Loomis | - | - |
| Play of the Week | Don Parritt | TV | - |
| Tate | John Torsett | TV | - |
| The Iceman Cometh | Don Parritt | TM | - |